hahn_1995 ========= J\. W\. Hahn and E\. S\. Lee, J\. Opt\. Soc\. Am\. B 12, 1021 \(1995\) `Source record `__ · :doc:`Catalogue ` · :doc:`Review register ` DOI: `10\.1364/josab\.12\.001021 `__ **Source kind:** measurement **Recorded technique:** Nonlinear interferometry of CARS\: two gas cells in series \(argon reference, sample\), with a phase\-shifting unit of sliding BK\-7 wedges between them; the fringe amplitude of the summed CARS signal against the sample pressure \(up to 2 bar, transducer calibrated to 0\.1 %\) gives the sample's nonresonant susceptibility relative to argon's\. BOXCARS phase matching, injection\-seeded single\-mode Nd\:YAG pump at 532 nm \(\< 100 MHz, 7\-8 ns\) and a single\-mode pulsed dye Stokes \(about 500 MHz\), Raman shift 2157 cm^\-1 \(2334 cm^\-1 for CO, CF4, H2\), parallel polarizations; shot\-by\-shot normalization to propane's nonresonant CARS\. **Materials in structured entries:** Ar, CH4, CO, CO2, H2, N2, O2 **Dataset quantities:** hyperpolarizability\_ratio, nonlinear\_susceptibility **Contents:** 53 datasets; 0 formulas. Curation notes -------------- Nonresonant CARS susceptibilities relative to argon, for C2H2, CO2, CH4, N2, O2, C3H8, CO, CF4 \('Freon'\) and H2; acetylene, propane and CF4 are not curated species \(skipped\)\. Definitions\: the CARS susceptibility of the CARS literature, Eq\. \(14\), p\. 1025 \(after Druet and Taran\)\: chi\_CARS\(3\) = \(N/hbar\) sum \(rho\_aa \- rho\_bb\) c^4/\(w1 w2^3\) \(d sigma/d Omega\) / \(w\_ba \- w1 \+ w2 \+ i gamma\_ba\), N the number density; the off\-resonant Raman part, Eq\. \(15\), neglects i gamma\. Values per amagat, 10^\-18 cm^3/\(erg amagat\)\. The absolute scale is argon's 9\.46 x 10^\-18 cm^3/\(erg amagat\) 'reported by Rosasco and Hurst' \(Table 1 note b\)\: rosasco\_1985's 3 sigma/24 = 0\.788 x 10^\-18 esu times 12 \(their chi^CARS = 12 chi\_1111\), the same convention as farrow\_1985\: chi^CARS = N0 gamma\_T/2 at 1 amagat, gamma\_T = 2 chi^CARS/N0 \(1e\-18 per amagat = 147\.8 au\)\. Eqs\. \(1\)\-\(13\) \(pp\. 1022\-1023\) model the interference\: I ~ 1 \+ eta^2 \+ 2 eta cos\(\.\.\.\), eta = chi\_s P\_s phi / \(chi\_r P\_r\); the fringe amplitude is linear in the sample pressure\. Results\: Table 1 \(p\. 1025\) ratio of fringe slopes to argon's \(uncertainty 'usually about 2\-3 % and \.\.\. no larger than 5 %', p\. 1025\) and effective chi\_NR \(ratio x 9\.46\); Table 2 \(p\. 1025\) the off\-resonant Raman terms computed from Eq\. \(15\) with Schrotter and Klockner's \(curated as schrotter\_1979\) and Martin's cross sections; Table 3 \(p\. 1026\) the electronic chi\_NR = effective minus off\-resonant \(checked\: CO2 10\.8 \+ 0\.35 \+ 0\.62 = 11\.77, CH4 26\.9 \- 4\.17 = 22\.73, N2 10\.2 \- 2\.30 = 7\.90, O2 7\.31 \+ 0\.67 = 7\.98, CO 10\.3 \+ 2\.03 = 12\.33, H2 6\.66 \- 0\.77 = 5\.89 against 5\.90 printed\)\. 'The uncertainties of the absolute values of the electronic susceptibility \.\.\. are estimated to be 10 %' \(Table 3 note a\); 'overall uncertainty \.\.\. is less than 5 %' \(abstract, conclusion; the relative measurement\)\. Check measurement \(p\. 1026\)\: O2 at 2334 cm^\-1, effective 7\.28 \+\- 0\.18, off\-resonant \-0\.53, electronic 7\.81 x 10^\-18, 2\.1 % from the 2157 cm^\-1 value\. Part\: the effective values contain the off\-resonant vibrational Raman tails at the measurement's Raman shift \(recorded total\); the electronic values subtract the computed tails \(the subtraction of computed gamma^v; no orientational term enters CARS at these detunings\)\. The library text of this paper has glyph errors \(10^\-18 as '10218', cm^\-1 as 'cm21', minus signs as '2'\); every value was read against the table images\. **Recorded bibliographic identity status:** VALIDATED\_WITH\_WARNINGS. This concerns identification of the source; it does not establish the scientific correctness of its contents. Datasets -------- hahn\_1995/electronic\_CO2 ~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "electronic_CO2", "material": "CO2", "file": "CO2/hahn_1995__electronic_CO2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "primary", "uncertainty": { "relative": 0.1, "level": "not stated" }, "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic", "raman_shift_cm1": 2157 } } Table 3 \(p\. 1026\), 'This Experiment'\: the electronic chi\_NR\(3\), Table 1's effective value minus Table 2's computed off\-resonant Raman term, per amagat, at the 532 nm pump and Raman shift 2157 cm^\-1; argon's 9\.46 \(Rosasco and Hurst\) is the scale\. Uncertainty 10 % absolute \(note a\)\. CARS chi^CARS convention \(gamma\_T = 2 chi/N0\)\. hahn\_1995/electronic\_CH4 ~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "electronic_CH4", "material": "CH4", "file": "CH4/hahn_1995__electronic_CH4.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "primary", "uncertainty": { "relative": 0.1, "level": "not stated" }, "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic", "raman_shift_cm1": 2157 } } Table 3 \(p\. 1026\), 'This Experiment'\: the electronic chi\_NR\(3\), Table 1's effective value minus Table 2's computed off\-resonant Raman term, per amagat, at the 532 nm pump and Raman shift 2157 cm^\-1; argon's 9\.46 \(Rosasco and Hurst\) is the scale\. Uncertainty 10 % absolute \(note a\)\. CARS chi^CARS convention \(gamma\_T = 2 chi/N0\)\. hahn\_1995/electronic\_N2 ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "electronic_N2", "material": "N2", "file": "N2/hahn_1995__electronic_N2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "primary", "uncertainty": { "relative": 0.1, "level": "not stated" }, "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic", "raman_shift_cm1": 2157 } } Table 3 \(p\. 1026\), 'This Experiment'\: the electronic chi\_NR\(3\), Table 1's effective value minus Table 2's computed off\-resonant Raman term, per amagat, at the 532 nm pump and Raman shift 2157 cm^\-1; argon's 9\.46 \(Rosasco and Hurst\) is the scale\. Uncertainty 10 % absolute \(note a\)\. CARS chi^CARS convention \(gamma\_T = 2 chi/N0\)\. hahn\_1995/electronic\_O2 ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "electronic_O2", "material": "O2", "file": "O2/hahn_1995__electronic_O2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "primary", "uncertainty": { "relative": 0.1, "level": "not stated" }, "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic", "raman_shift_cm1": 2157 } } Table 3 \(p\. 1026\), 'This Experiment'\: the electronic chi\_NR\(3\), Table 1's effective value minus Table 2's computed off\-resonant Raman term, per amagat, at the 532 nm pump and Raman shift 2157 cm^\-1; argon's 9\.46 \(Rosasco and Hurst\) is the scale\. Uncertainty 10 % absolute \(note a\)\. CARS chi^CARS convention \(gamma\_T = 2 chi/N0\)\. hahn\_1995/electronic\_CO ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "electronic_CO", "material": "CO", "file": "CO/hahn_1995__electronic_CO.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "primary", "uncertainty": { "relative": 0.1, "level": "not stated" }, "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic", "raman_shift_cm1": 2334 } } Table 3 \(p\. 1026\), 'This Experiment'\: the electronic chi\_NR\(3\), Table 1's effective value minus Table 2's computed off\-resonant Raman term, per amagat, at the 532 nm pump and Raman shift 2334 cm^\-1; argon's 9\.46 \(Rosasco and Hurst\) is the scale\. Uncertainty 10 % absolute \(note a\)\. CARS chi^CARS convention \(gamma\_T = 2 chi/N0\)\. hahn\_1995/electronic\_H2 ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "electronic_H2", "material": "H2", "file": "H2/hahn_1995__electronic_H2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "primary", "uncertainty": { "relative": 0.1, "level": "not stated" }, "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic", "raman_shift_cm1": 2334 } } Table 3 \(p\. 1026\), 'This Experiment'\: the electronic chi\_NR\(3\), Table 1's effective value minus Table 2's computed off\-resonant Raman term, per amagat, at the 532 nm pump and Raman shift 2334 cm^\-1; argon's 9\.46 \(Rosasco and Hurst\) is the scale\. Uncertainty 10 % absolute \(note a\)\. CARS chi^CARS convention \(gamma\_T = 2 chi/N0\)\. hahn\_1995/effective\_CO2 ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "effective_CO2", "material": "CO2", "file": "CO2/hahn_1995__effective_CO2.csv", "table": "tbl_50a8b1a2127a", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "uncertainty": { "column": true, "level": "not stated" }, "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "total", "raman_shift_cm1": 2157 } } Table 1 \(p\. 1025\), effective chi\_NR\(3\) \(the row is the Raman shift in cm^\-1\), the fringe\-slope ratio times argon's 9\.46 \(note b\); parenthesized uncertainty\. Includes the off\-resonant Raman tail at this shift\: total\. Not independent of ratio\_ and electronic\_\. hahn\_1995/effective\_CH4 ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "effective_CH4", "material": "CH4", "file": "CH4/hahn_1995__effective_CH4.csv", "table": "tbl_50a8b1a2127a", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "uncertainty": { "column": true, "level": "not stated" }, "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "total", "raman_shift_cm1": 2157 } } Table 1 \(p\. 1025\), effective chi\_NR\(3\) \(the row is the Raman shift in cm^\-1\), the fringe\-slope ratio times argon's 9\.46 \(note b\); parenthesized uncertainty\. Includes the off\-resonant Raman tail at this shift\: total\. Not independent of ratio\_ and electronic\_\. hahn\_1995/effective\_N2 ~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "effective_N2", "material": "N2", "file": "N2/hahn_1995__effective_N2.csv", "table": "tbl_50a8b1a2127a", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "uncertainty": { "column": true, "level": "not stated" }, "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "total", "raman_shift_cm1": 2157 } } Table 1 \(p\. 1025\), effective chi\_NR\(3\) \(the row is the Raman shift in cm^\-1\), the fringe\-slope ratio times argon's 9\.46 \(note b\); parenthesized uncertainty\. Includes the off\-resonant Raman tail at this shift\: total\. Not independent of ratio\_ and electronic\_\. hahn\_1995/effective\_O2 ~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "effective_O2", "material": "O2", "file": "O2/hahn_1995__effective_O2.csv", "table": "tbl_50a8b1a2127a", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "uncertainty": { "column": true, "level": "not stated" }, "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "total", "raman_shift_cm1": 2157 } } Table 1 \(p\. 1025\), effective chi\_NR\(3\) \(the row is the Raman shift in cm^\-1\), the fringe\-slope ratio times argon's 9\.46 \(note b\); parenthesized uncertainty\. Includes the off\-resonant Raman tail at this shift\: total\. Not independent of ratio\_ and electronic\_\. hahn\_1995/effective\_CO ~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "effective_CO", "material": "CO", "file": "CO/hahn_1995__effective_CO.csv", "table": "tbl_50a8b1a2127a", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "uncertainty": { "column": true, "level": "not stated" }, "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "total", "raman_shift_cm1": 2334 } } Table 1 \(p\. 1025\), effective chi\_NR\(3\) \(the row is the Raman shift in cm^\-1\), the fringe\-slope ratio times argon's 9\.46 \(note b\); parenthesized uncertainty\. Includes the off\-resonant Raman tail at this shift\: total\. Not independent of ratio\_ and electronic\_\. hahn\_1995/effective\_H2 ~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "effective_H2", "material": "H2", "file": "H2/hahn_1995__effective_H2.csv", "table": "tbl_50a8b1a2127a", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "uncertainty": { "column": true, "level": "not stated" }, "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "total", "raman_shift_cm1": 2334 } } Table 1 \(p\. 1025\), effective chi\_NR\(3\) \(the row is the Raman shift in cm^\-1\), the fringe\-slope ratio times argon's 9\.46 \(note b\); parenthesized uncertainty\. Includes the off\-resonant Raman tail at this shift\: total\. Not independent of ratio\_ and electronic\_\. hahn\_1995/ratio\_CO2 ~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "ratio_CO2", "material": "CO2", "file": "CO2/hahn_1995__ratio_CO2.csv", "table": "tbl_50a8b1a2127a", "quantity": "hyperpolarizability_ratio", "abscissa_unit": "nm", "use": "check", "uncertainty": { "column": true, "level": "not stated" }, "parameters": { "reference_material": "Ar", "process": "cars", "part": "total", "raman_shift_cm1": 2157 } } Table 1 \(p\. 1025\), 'Ratio of the slope of the interference fringe of the sample gas to that of argon' \(note a; row = Raman shift in cm^\-1\)\: the measured ratio of the effective CARS susceptibilities at equal density \(the ratio of the effective gammas\), the paper's primary measurement; uncertainty in parentheses\. Effective\: includes the off\-resonant Raman tail \(total\)\. hahn\_1995/ratio\_CH4 ~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "ratio_CH4", "material": "CH4", "file": "CH4/hahn_1995__ratio_CH4.csv", "table": "tbl_50a8b1a2127a", "quantity": "hyperpolarizability_ratio", "abscissa_unit": "nm", "use": "check", "uncertainty": { "column": true, "level": "not stated" }, "parameters": { "reference_material": "Ar", "process": "cars", "part": "total", "raman_shift_cm1": 2157 } } Table 1 \(p\. 1025\), 'Ratio of the slope of the interference fringe of the sample gas to that of argon' \(note a; row = Raman shift in cm^\-1\)\: the measured ratio of the effective CARS susceptibilities at equal density \(the ratio of the effective gammas\), the paper's primary measurement; uncertainty in parentheses\. Effective\: includes the off\-resonant Raman tail \(total\)\. hahn\_1995/ratio\_N2 ~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "ratio_N2", "material": "N2", "file": "N2/hahn_1995__ratio_N2.csv", "table": "tbl_50a8b1a2127a", "quantity": "hyperpolarizability_ratio", "abscissa_unit": "nm", "use": "check", "uncertainty": { "column": true, "level": "not stated" }, "parameters": { "reference_material": "Ar", "process": "cars", "part": "total", "raman_shift_cm1": 2157 } } Table 1 \(p\. 1025\), 'Ratio of the slope of the interference fringe of the sample gas to that of argon' \(note a; row = Raman shift in cm^\-1\)\: the measured ratio of the effective CARS susceptibilities at equal density \(the ratio of the effective gammas\), the paper's primary measurement; uncertainty in parentheses\. Effective\: includes the off\-resonant Raman tail \(total\)\. hahn\_1995/ratio\_O2 ~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "ratio_O2", "material": "O2", "file": "O2/hahn_1995__ratio_O2.csv", "table": "tbl_50a8b1a2127a", "quantity": "hyperpolarizability_ratio", "abscissa_unit": "nm", "use": "check", "uncertainty": { "column": true, "level": "not stated" }, "parameters": { "reference_material": "Ar", "process": "cars", "part": "total", "raman_shift_cm1": 2157 } } Table 1 \(p\. 1025\), 'Ratio of the slope of the interference fringe of the sample gas to that of argon' \(note a; row = Raman shift in cm^\-1\)\: the measured ratio of the effective CARS susceptibilities at equal density \(the ratio of the effective gammas\), the paper's primary measurement; uncertainty in parentheses\. Effective\: includes the off\-resonant Raman tail \(total\)\. hahn\_1995/ratio\_CO ~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "ratio_CO", "material": "CO", "file": "CO/hahn_1995__ratio_CO.csv", "table": "tbl_50a8b1a2127a", "quantity": "hyperpolarizability_ratio", "abscissa_unit": "nm", "use": "check", "uncertainty": { "column": true, "level": "not stated" }, "parameters": { "reference_material": "Ar", "process": "cars", "part": "total", "raman_shift_cm1": 2334 } } Table 1 \(p\. 1025\), 'Ratio of the slope of the interference fringe of the sample gas to that of argon' \(note a; row = Raman shift in cm^\-1\)\: the measured ratio of the effective CARS susceptibilities at equal density \(the ratio of the effective gammas\), the paper's primary measurement; uncertainty in parentheses\. Effective\: includes the off\-resonant Raman tail \(total\)\. hahn\_1995/ratio\_H2 ~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "ratio_H2", "material": "H2", "file": "H2/hahn_1995__ratio_H2.csv", "table": "tbl_50a8b1a2127a", "quantity": "hyperpolarizability_ratio", "abscissa_unit": "nm", "use": "check", "uncertainty": { "column": true, "level": "not stated" }, "parameters": { "reference_material": "Ar", "process": "cars", "part": "total", "raman_shift_cm1": 2334 } } Table 1 \(p\. 1025\), 'Ratio of the slope of the interference fringe of the sample gas to that of argon' \(note a; row = Raman shift in cm^\-1\)\: the measured ratio of the effective CARS susceptibilities at equal density \(the ratio of the effective gammas\), the paper's primary measurement; uncertainty in parentheses\. Effective\: includes the off\-resonant Raman tail \(total\)\. hahn\_1995/off\_resonant\_CO2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "off_resonant_CO2", "material": "CO2", "file": "CO2/hahn_1995__off_resonant_CO2.csv", "table": "tbl_4564b15b3033", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "vibrational", "raman_shift_cm1": 2157 } } Table 2 \(p\. 1025\), the calculated off\-resonant Raman term \(Eq\. \(15\)\) at the measurement's Raman shift; rows are the Raman bands in cm^\-1\: rows 1285 and 1388 \(the two Fermi\-dyad bands\), \-0\.35 and \-0\.62\. The library lost the minus signs \(restored in the extraction script from the image\)\. Computed, vibrational \(Q\-branch\) Raman tails; specific to the Raman shift\. hahn\_1995/off\_resonant\_CH4 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "off_resonant_CH4", "material": "CH4", "file": "CH4/hahn_1995__off_resonant_CH4.csv", "table": "tbl_4564b15b3033", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "vibrational", "raman_shift_cm1": 2157 } } Table 2 \(p\. 1025\), the calculated off\-resonant Raman term \(Eq\. \(15\)\) at the measurement's Raman shift; rows are the Raman bands in cm^\-1\: row 2917, \+4\.17\. The library lost the minus signs \(restored in the extraction script from the image\)\. Computed, vibrational \(Q\-branch\) Raman tails; specific to the Raman shift\. hahn\_1995/off\_resonant\_N2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "off_resonant_N2", "material": "N2", "file": "N2/hahn_1995__off_resonant_N2.csv", "table": "tbl_4564b15b3033", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "vibrational", "raman_shift_cm1": 2157 } } Table 2 \(p\. 1025\), the calculated off\-resonant Raman term \(Eq\. \(15\)\) at the measurement's Raman shift; rows are the Raman bands in cm^\-1\: row 2331, \+2\.30\. The library lost the minus signs \(restored in the extraction script from the image\)\. Computed, vibrational \(Q\-branch\) Raman tails; specific to the Raman shift\. hahn\_1995/off\_resonant\_O2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "off_resonant_O2", "material": "O2", "file": "O2/hahn_1995__off_resonant_O2.csv", "table": "tbl_4564b15b3033", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "vibrational", "raman_shift_cm1": 2157 } } Table 2 \(p\. 1025\), the calculated off\-resonant Raman term \(Eq\. \(15\)\) at the measurement's Raman shift; rows are the Raman bands in cm^\-1\: row 1555, \-0\.67\. The library lost the minus signs \(restored in the extraction script from the image\)\. Computed, vibrational \(Q\-branch\) Raman tails; specific to the Raman shift\. hahn\_1995/off\_resonant\_CO ~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "off_resonant_CO", "material": "CO", "file": "CO/hahn_1995__off_resonant_CO.csv", "table": "tbl_4564b15b3033", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "vibrational", "raman_shift_cm1": 2334 } } Table 2 \(p\. 1025\), the calculated off\-resonant Raman term \(Eq\. \(15\)\) at the measurement's Raman shift; rows are the Raman bands in cm^\-1\: row 2143, \-2\.03 \(at 2334 cm^\-1\)\. The library lost the minus signs \(restored in the extraction script from the image\)\. Computed, vibrational \(Q\-branch\) Raman tails; specific to the Raman shift\. hahn\_1995/off\_resonant\_H2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "off_resonant_H2", "material": "H2", "file": "H2/hahn_1995__off_resonant_H2.csv", "table": "tbl_4564b15b3033", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "vibrational", "raman_shift_cm1": 2334 } } Table 2 \(p\. 1025\), the calculated off\-resonant Raman term \(Eq\. \(15\)\) at the measurement's Raman shift; rows are the Raman bands in cm^\-1\: row 4156, \+0\.77 \(at 2334 cm^\-1\)\. The library lost the minus signs \(restored in the extraction script from the image\)\. Computed, vibrational \(Q\-branch\) Raman tails; specific to the Raman shift\. hahn\_1995/electronic\_2334\_O2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "electronic_2334_O2", "material": "O2", "table": "text", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "use": "check", "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic", "raman_shift_cm1": 2334 } } 1 inline points in the source record. p\. 1026\: O2 remeasured at the 2334 cm^\-1 Raman shift\: effective 7\.28 x 10^\-18 \+\- 0\.18, off\-resonant \-0\.53 x 10^\-18, electronic 7\.81 x 10^\-18 cm^3/\(erg amagat\), 'which differs by only 2\.1 % from the value listed in Table 3' \(7\.98 at 2157 cm^\-1\)\. A consistency check\. hahn\_1995/irs\_rosasco\_hurst\_Ar ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "irs_rosasco_hurst_Ar", "material": "Ar", "file": "Ar/hahn_1995__irs_rosasco_hurst_Ar.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "standard_air", "use": "reproduced", "reproduced_from": [ "rosasco_1985" ], "parameters": { "process": "kerr", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column IRS \(676 \+ 584 nm, note b\: Refs\. 23 and 28, Rosasco and Hurst 1985, 1986\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Checked\: 12 x 0\.788 = 9\.46\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/irs\_rosasco\_hurst\_H2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "irs_rosasco_hurst_H2", "material": "H2", "file": "H2/hahn_1995__irs_rosasco_hurst_H2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "standard_air", "use": "reproduced", "reproduced_from": [ "rosasco_1986" ], "parameters": { "process": "kerr", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column IRS \(676 \+ 584 nm, note b\: Refs\. 23 and 28, Rosasco and Hurst 1985, 1986\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Checked\: 12 x 1\.5 x 0\.2966 = 5\.34\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_farrow\_Ar ~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_farrow_Ar", "material": "Ar", "file": "Ar/hahn_1995__cars_farrow_Ar.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "farrow_1985" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 607 nm, note c\: Refs\. 15 and 25, Farrow and Rahn 1985, Farrow et al\. 1987\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_farrow\_N2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_farrow_N2", "material": "N2", "file": "N2/hahn_1995__cars_farrow_N2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "farrow_1985" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 607 nm, note c\: Refs\. 15 and 25, Farrow and Rahn 1985, Farrow et al\. 1987\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/eshg\_shelton\_rice\_Ar ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "eshg_shelton_rice_Ar", "material": "Ar", "file": "Ar/hahn_1995__eshg_shelton_rice_Ar.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "shelton_1994" ], "parameters": { "process": "eshg", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column EHSG \[sic\] \(694 nm, note d\: 'static electric\-field\-induced second\-harmonic generation, Ref\. 42', Shelton and Rice 1994\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/eshg\_shelton\_rice\_CO2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "eshg_shelton_rice_CO2", "material": "CO2", "file": "CO2/hahn_1995__eshg_shelton_rice_CO2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "shelton_1994" ], "parameters": { "process": "eshg", "convention": "chi_cars_per_amagat", "part": "total" } } Table 3 \(p\. 1026\), column EHSG \[sic\] \(694 nm, note d\: 'static electric\-field\-induced second\-harmonic generation, Ref\. 42', Shelton and Rice 1994\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/eshg\_shelton\_rice\_CH4 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "eshg_shelton_rice_CH4", "material": "CH4", "file": "CH4/hahn_1995__eshg_shelton_rice_CH4.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "shelton_1994" ], "parameters": { "process": "eshg", "convention": "chi_cars_per_amagat", "part": "total" } } Table 3 \(p\. 1026\), column EHSG \[sic\] \(694 nm, note d\: 'static electric\-field\-induced second\-harmonic generation, Ref\. 42', Shelton and Rice 1994\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/eshg\_shelton\_rice\_N2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "eshg_shelton_rice_N2", "material": "N2", "file": "N2/hahn_1995__eshg_shelton_rice_N2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "shelton_1994" ], "parameters": { "process": "eshg", "convention": "chi_cars_per_amagat", "part": "total" } } Table 3 \(p\. 1026\), column EHSG \[sic\] \(694 nm, note d\: 'static electric\-field\-induced second\-harmonic generation, Ref\. 42', Shelton and Rice 1994\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/eshg\_shelton\_rice\_O2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "eshg_shelton_rice_O2", "material": "O2", "file": "O2/hahn_1995__eshg_shelton_rice_O2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "shelton_1994" ], "parameters": { "process": "eshg", "convention": "chi_cars_per_amagat", "part": "total" } } Table 3 \(p\. 1026\), column EHSG \[sic\] \(694 nm, note d\: 'static electric\-field\-induced second\-harmonic generation, Ref\. 42', Shelton and Rice 1994\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/eshg\_shelton\_rice\_CO ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "eshg_shelton_rice_CO", "material": "CO", "file": "CO/hahn_1995__eshg_shelton_rice_CO.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "shelton_1994" ], "parameters": { "process": "eshg", "convention": "chi_cars_per_amagat", "part": "total" } } Table 3 \(p\. 1026\), column EHSG \[sic\] \(694 nm, note d\: 'static electric\-field\-induced second\-harmonic generation, Ref\. 42', Shelton and Rice 1994\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/eshg\_shelton\_rice\_H2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "eshg_shelton_rice_H2", "material": "H2", "file": "H2/hahn_1995__eshg_shelton_rice_H2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "shelton_1994" ], "parameters": { "process": "eshg", "convention": "chi_cars_per_amagat", "part": "total" } } Table 3 \(p\. 1026\), column EHSG \[sic\] \(694 nm, note d\: 'static electric\-field\-induced second\-harmonic generation, Ref\. 42', Shelton and Rice 1994\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_used\_CO2 ~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_used_CO2", "material": "CO2", "file": "CO2/hahn_1995__cars_used_CO2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "unattributed in the paper (Table 3 note e); possibly B. Lange and J. Wolfrum, Appl. Phys. B 51, 53 (1990)" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 683 nm, note e\: 'Effective chi\_NR obtained by comparing the absolute intensities of the nonresonant CARS signals of two gases in a USED CARS configuration'; no reference is given \(the paper's otherwise uncited Ref\. 43, Lange and Wolfrum, is on USED CARS\)\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_used\_CH4 ~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_used_CH4", "material": "CH4", "file": "CH4/hahn_1995__cars_used_CH4.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "unattributed in the paper (Table 3 note e); possibly B. Lange and J. Wolfrum, Appl. Phys. B 51, 53 (1990)" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 683 nm, note e\: 'Effective chi\_NR obtained by comparing the absolute intensities of the nonresonant CARS signals of two gases in a USED CARS configuration'; no reference is given \(the paper's otherwise uncited Ref\. 43, Lange and Wolfrum, is on USED CARS\)\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_used\_N2 ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_used_N2", "material": "N2", "file": "N2/hahn_1995__cars_used_N2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "unattributed in the paper (Table 3 note e); possibly B. Lange and J. Wolfrum, Appl. Phys. B 51, 53 (1990)" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 683 nm, note e\: 'Effective chi\_NR obtained by comparing the absolute intensities of the nonresonant CARS signals of two gases in a USED CARS configuration'; no reference is given \(the paper's otherwise uncited Ref\. 43, Lange and Wolfrum, is on USED CARS\)\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_used\_O2 ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_used_O2", "material": "O2", "file": "O2/hahn_1995__cars_used_O2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "unattributed in the paper (Table 3 note e); possibly B. Lange and J. Wolfrum, Appl. Phys. B 51, 53 (1990)" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 683 nm, note e\: 'Effective chi\_NR obtained by comparing the absolute intensities of the nonresonant CARS signals of two gases in a USED CARS configuration'; no reference is given \(the paper's otherwise uncited Ref\. 43, Lange and Wolfrum, is on USED CARS\)\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_used\_H2 ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_used_H2", "material": "H2", "file": "H2/hahn_1995__cars_used_H2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "unattributed in the paper (Table 3 note e); possibly B. Lange and J. Wolfrum, Appl. Phys. B 51, 53 (1990)" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 683 nm, note e\: 'Effective chi\_NR obtained by comparing the absolute intensities of the nonresonant CARS signals of two gases in a USED CARS configuration'; no reference is given \(the paper's otherwise uncited Ref\. 43, Lange and Wolfrum, is on USED CARS\)\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_lundeen\_Ar ~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_lundeen_Ar", "material": "Ar", "file": "Ar/hahn_1995__cars_lundeen_Ar.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "lundeen_1983" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 683 nm, note f\: Ref\. 22, Lundeen et al\.\)\: 3 x Lundeen's per\-molecule chi x 2\.687e19; per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Checked\: 131 \-\> 10\.56\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_lundeen\_CO2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_lundeen_CO2", "material": "CO2", "file": "CO2/hahn_1995__cars_lundeen_CO2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "lundeen_1983" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 683 nm, note f\: Ref\. 22, Lundeen et al\.\)\: 3 x Lundeen's per\-molecule chi x 2\.687e19; per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Checked\: 153 \-\> 12\.33\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_lundeen\_CH4 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_lundeen_CH4", "material": "CH4", "file": "CH4/hahn_1995__cars_lundeen_CH4.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "lundeen_1983" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 683 nm, note f\: Ref\. 22, Lundeen et al\.\)\: 3 x Lundeen's per\-molecule chi x 2\.687e19; per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Checked\: 330 \-\> 26\.6\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_lundeen\_N2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_lundeen_N2", "material": "N2", "file": "N2/hahn_1995__cars_lundeen_N2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "lundeen_1983" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 683 nm, note f\: Ref\. 22, Lundeen et al\.\)\: 3 x Lundeen's per\-molecule chi x 2\.687e19; per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Checked\: 105 \-\> 8\.46\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_lundeen\_O2 ~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_lundeen_O2", "material": "O2", "file": "O2/hahn_1995__cars_lundeen_O2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "lundeen_1983" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 683 nm, note f\: Ref\. 22, Lundeen et al\.\)\: 3 x Lundeen's per\-molecule chi x 2\.687e19; per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Checked\: 141 \-\> 11\.37\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_lundeen\_CO ~~~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_lundeen_CO", "material": "CO", "file": "CO/hahn_1995__cars_lundeen_CO.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "lundeen_1983" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(532 \+ 683 nm, note f\: Ref\. 22, Lundeen et al\.\)\: 3 x Lundeen's per\-molecule chi x 2\.687e19; per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Checked\: 155 \-\> 12\.49\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_rado\_Ar ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_rado_Ar", "material": "Ar", "file": "Ar/hahn_1995__cars_rado_Ar.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "rosasco_1985", "W. G. Rado, Appl. Phys. Lett. 11, 123 (1967)" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(694 \+ 976 nm, note g\: 'Ref\. 21 \[Rado\], reevaluated data; see text', with Rosasco and Hurst's H2 Q\(1\) value\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Checked\: 12 x 0\.776 = 9\.31 \(rosasco\_1985\)\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_rado\_CO2 ~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_rado_CO2", "material": "CO2", "file": "CO2/hahn_1995__cars_rado_CO2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "rosasco_1985", "W. G. Rado, Appl. Phys. Lett. 11, 123 (1967)" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(694 \+ 976 nm, note g\: 'Ref\. 21 \[Rado\], reevaluated data; see text', with Rosasco and Hurst's H2 Q\(1\) value\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_rado\_CH4 ~~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_rado_CH4", "material": "CH4", "file": "CH4/hahn_1995__cars_rado_CH4.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "rosasco_1985", "W. G. Rado, Appl. Phys. Lett. 11, 123 (1967)" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(694 \+ 976 nm, note g\: 'Ref\. 21 \[Rado\], reevaluated data; see text', with Rosasco and Hurst's H2 Q\(1\) value\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Checked\: 12 x 1\.48 = 17\.76, printed 17\.72\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_rado\_N2 ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_rado_N2", "material": "N2", "file": "N2/hahn_1995__cars_rado_N2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "rosasco_1985", "W. G. Rado, Appl. Phys. Lett. 11, 123 (1967)" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(694 \+ 976 nm, note g\: 'Ref\. 21 \[Rado\], reevaluated data; see text', with Rosasco and Hurst's H2 Q\(1\) value\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Checked\: 12 x 0\.676 = 8\.11\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_rado\_O2 ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_rado_O2", "material": "O2", "file": "O2/hahn_1995__cars_rado_O2.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "rosasco_1985", "W. G. Rado, Appl. Phys. Lett. 11, 123 (1967)" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(694 \+ 976 nm, note g\: 'Ref\. 21 \[Rado\], reevaluated data; see text', with Rosasco and Hurst's H2 Q\(1\) value\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Checked\: 12 x 0\.651 = 7\.81\. Reproduced and rescaled; about 10 % \(note a\)\. hahn\_1995/cars\_rado\_CO ~~~~~~~~~~~~~~~~~~~~~~~~~ .. code-block:: text { "id": "cars_rado_CO", "material": "CO", "file": "CO/hahn_1995__cars_rado_CO.csv", "table": "tbl_c1933c977eba", "quantity": "nonlinear_susceptibility", "unit": "cm3/(erg amagat)", "scale": 1e-18, "abscissa_unit": "nm", "wavelength_medium": "vacuum", "use": "reproduced", "reproduced_from": [ "rosasco_1985", "W. G. Rado, Appl. Phys. Lett. 11, 123 (1967)" ], "parameters": { "process": "cars", "convention": "chi_cars_per_amagat", "part": "electronic" } } Table 3 \(p\. 1026\), column CARS \(694 \+ 976 nm, note g\: 'Ref\. 21 \[Rado\], reevaluated data; see text', with Rosasco and Hurst's H2 Q\(1\) value\); per amagat, in the paper's chi^CARS units \(10^\-18 cm^3/\(erg amagat\)\), wavelength as the column header\. Reproduced and rescaled; about 10 % \(note a\)\. Formulas -------- No formulas are recorded. Corrections ----------- No dataset errata are recorded in this source record. Formula corrections, where recorded, appear with their formulas above. Curation notes may also discuss corrections or unresolved interpretation. Consult the :doc:`review register ` for the checks and decisions.